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Publication Title | Key Principles of Heterogeneous Catalysis

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Contents Preface XVII

List of Contributors XXI

1 Molecular Catalytic Kinetics Concepts 1 Rutger A. van Santen

1.1 Key Principles of Heterogeneous Catalysis 1

1.2 Elementary Rate Constants and Catalytic Cycle 1

1.3 Linear Activation Energy – Reaction Energy Relationships

1.4 Microkinetic Expressions; Derivation of Volcano Curve

1.5 Compensation Effect 12

1.6 Hydrocarbon Conversion Catalyzed by Zeolites 14

1.7 Structure Sensitive and Insensitive Reactions 17

1.8 The Nonmetal Atom Sharing Rule of Low-Barrier Transition

States 22

1.8.1 Introduction 22

1.8.2 Ammonia Oxidation 24

1.9 Summary 29

References 29

2 Hierarchical Porous Zeolites by Demetallation 31 Johan C. Groen and Javier Pe ́rez-Ram ́ırez

2.1 Zeolites and Catalyst Effectiveness 31

2.2 Hierarchical Zeolites 33

2.3 Mesoporous Zeolites by Demetallation 34

2.4 Desilication 36

2.4.1 Introduction 36

2.4.2 Role of the Trivalent Cation 37

2.4.2.1 Framework Aluminum 37

2.4.2.2 Nonframework Aluminum 38

2.4.2.3 Distribution of Aluminum in the Framework 39

2.4.2.4 Different Zeolite Framework Topologies 39

2.4.2.5 Framework Trivalent Cations Different from Aluminum 40

Novel Concepts in Catalysis and Chemical Reactors: Improving the Efficiency for the Future. Edited by Andrzej Cybulski, Jacob A. Moulijn, and Andrzej Stankiewicz

Copyright  2010 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim

ISBN: 978-3-527-32469-9

2 6

VII

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